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iOS Design Kit - The newest library of native iOS templates
Xcode - Xcode is Apple’s powerful integrated development environment for creating great apps for Mac, iPhone, and iPad. Xcode 4 includes the Xcode IDE, instruments, iOS Simulator, and the latest Mac OS X and iOS SDKs.
draw.io - Online diagramming application
Pencil Project - Single-user mockup / wireframing / diagramming tool
Angle 2 Mockups - A giant Sketch Library for creating app presentations
quickMockup - Online tool for creating mockups in the browser.